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It's a text string, so it's sorting as text.
You either need to split it to a number field so it can sort as a number, or add leading zeros to the 1-9 values.
Yes, or possibly 'Show value only from second field' & 'Sort values using First field' in the Specify Fields for Value List dialog.
(not tested, as I don't know your fields or your value list set up)
Need adding on 1-99 as the value could be 100, and leading character can be space if want.