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If you want to base your chart on a found set of records (which can be all records or whatever you pull up via a Find or GTRR), You can use a "count of" summary field to get a count of each type of lead origin.
Make the Lead Origin Field the data source for your x-series
Make the summary field the data source for the y-series
Sort your records by Lead Origin
Make sure that your data source options for the chart object specify "summarized data".
If you want a pie chart, use a "fraction of total" summary field.
And you can only sort on the Lead Origin Field. Sorting on multiple fields can screw up your chart. If that's an issue, you may need to either use different methods or add a calculation field that combines data from several fields in such a way that you can sort on that one field to get your chart in place of sorting on the multiple fields.